By Eliezer Gileadi
Supplying an intensive rationalization of electrode kinetics, this textbook emphasizes actual phenomena-rather than mathematical formalism-and elucidates the underlying ideas of the various experimental recommendations. Assuming an hassle-free wisdom of thermodynamics and chemical kinetics and minimum mathematical talents, insurance explores the arguments of 2 basic colleges of proposal: electrode kinetics and interfacial electrochemistry considered as a department of actual chemistry, and from the point of view of analytical chemistry.
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Additional info for Electrode Kinetics for Chemists, Chemical Engineers and Materials Scientists
Bossel, Final Report on SOFC Data Facts and Figures, Berne, CH: Swiss Federal Oﬃce of Energy, 1992. 14. J. V. Virkar, K. Fung, K. C. Singhal, Polarization eﬀects in intermediate temperature, anode-supportedsolid oxide fuel cells, J. Electrochem. Soc, 1999, 146(1), 69–78. 15. C. O. Colpan, F. Hamdullahpur and I. Dincer, Heat-up and start-up modeling of direct internal reforming solid oxide fuel cells, J. Power Sources, 2010, 195, 3579–3589. 16. E. Achenbach, SOFC Stack Modelling, Final Report Of Activity A2, Annex II: Modelling and Evaluation of Advanced Solid Oxide Fuel Cells, International Energy Agency Programme on R, D&D on Advanced Fuel Cells, Juelich, Germany, 1996.
15 O cm2,1 which can be reached for conventional yttria stabilized zirconia electrolyte with a membrane thickness of 15 mm at 700 1C. In practice, an operation temperature of 1000 1C was selected for Westinghouse’s cathode-supported tubular cell with YSZ electrolyte membrane thickness of 30–40 mm. High operating temperature, RSC Energy and Environment Series No. 7 Solid Oxide Fuel Cells: From Materials to System Modeling Edited by Meng Ni and Tim S. org 26 View Online on 01/09/2013 10:28:55. 1039/9781849737777-00026 Electrolyte Materials for Solid Oxide Fuel Cells (SOFCs) 27 however, has become a major obstacle for the widespread application of SOFC technology because of the related high costs, long start-up times, low long-term security and poor portability.
Katahira et al. 2O3Àd series, was studied by Zuo et al. 166 However, later experiments illustrated that BZCY1 still had insuﬃcient stability under a reforming gas atmosphere. Fabbri et al. 170 The optimal Zr doping content was around 40–50% of the B-site cations. 2O3Àd electrolyte-supported cell delivered a PPD of only 18 mW cmÀ2 at 700 1C. A synergetic eﬀect between the electrode and electrolyte was created. The participation of Zr and Zn eﬀectively enhanced the chemical stability with no vital deterioration on the protonic conductivity.
Electrode Kinetics for Chemists, Chemical Engineers and Materials Scientists by Eliezer Gileadi